Noriko Yamaguchi1, Katsutoshi Seki2, Misako Komamura1, and Hideshi Fujiwara1. (1) National Institute for Agro-Environmental Sciences, 3-1-3, Kan-nondai, Tsukuba Ibaraki, 305-8604, Japan, (2) The University of Tokyo, 1-1-1, Yayoi, Bunkyo, Tokyo, 113-8657, Japan
Atmospheric nuclear tests from 1945 to 1980 distributed radioactive fallout all over the world. Since 1959, we have monitored the concentrations of 137Cs and 90Sr in the plowed layer of paddy and upland soils collected annually from 17 agricultural fields in Japan. In the plowed layer of agricultural soils, the concentrations of 137Cs and 90Sr tended to decrease after 1964, although these concentrations varied through the years until 1980, in conjunction with the scale and frequency of atmospheric nuclear tests. The decreased concentrations of 137Cs and 90Sr were attributed to radioactive decay and downward migration. The decreasing rates of 137Cs that remained in the plowed layer were higher than those of 90Sr both in paddy and upland soils. This was because 90Sr leached from soil more readily than 137Cs. 137Cs was more likely to remain in upland soil than in paddy soil. The apparent residence half-time of 137Cs and 90Sr in the plowed layer at each sampling site was calculated by exponential regression of the monitoring data after 1964. A principal component analysis was performed on the soil physico-chemical properties. The extracted first principal component (PC1) was related to the sorption characteristics of soils. The reciprocal residence half-time of 137Cs and 90Sr in the plowed layer of upland soils was related to PC1 and the mean annual precipitation amounts. In conclusion, major factors in determining the decrease of 137Cs and 90Sr from the plowed layer were the soil sorption characteristics and precipitation amounts in the upland field.
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